najoNanosystems: Physics, Chemistry, MathematicsНаносистемы: физика, химия, математика2220-80542305-7971Университет ИТМО10.17586/2220-8054-2018-9-5-641-662najo-742Research ArticleCHEMISTRY AND MATERIALS SCIENCEХИМИЯ И НАУКА О МАТЕРИАЛАХThermodynamics and kinetics of non-autonomous phase formation in nanostructured materials with variable functional propertiesKovalenkoA. N.

26 Politekhnicheskaya, St. Petersburg 194021

ras-kan@mail.ruTugovaE. A.

26 Politekhnicheskaya, St. Petersburg 194021; ul. Professora Popova 5, St. Petersburg 197376

katugova@inbox.ruIoffe InstituteRussian FederationIoffe Institute; St. Petersburg Electrotechnical University “LETI”Russian Federation20181208202595641662Copyright © Kovalenko A.N., Tugova E.A., 20252025Kovalenko A.N., Tugova E.A.Kovalenko A.N., Tugova E.A.Данная работа распространяется под лицензией Creative Commons Attribution 4.0.This work is licensed under a Creative Commons Attribution 4.0 License.https://nanojournal.ifmo.ru/jour/article/view/742

The review addresses physico-chemical aspects of interaction between macro-, micro- and nano- structured units of matter with the analysis of interface and grain boundary entities (nonautonomous phases) mechanisms and formation, as well as methods of their control in order to achieve the desired functional properties of nanostructured materials. Construction of these materials involves identification of thermodynamic and kinetic regularities in the organization processes, state and genesis parameters of nonautonomous phases formed as specific nanosized structures in a limited space between the macroscopic volume phases and with the limited amount of substance, which differ significantly on their properties, structure and composition from the appropriate characteristics of volume phases. Studying them is based on the application and development of theoretical and experimental methods of non-equilibrium thermodynamics, chemical kinetics, nonlinear dynamics and fractal analysis to determine the conditions of self-organization or materials directed synthesis with a high content of nonautonomous phases. 

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The authors declare that there are no conflicts of interest present.