НАНОСИСТЕМЫ: ФИЗИКА, ХИМИЯ, МАТЕМАТИКА, 2011, 2 (1), С. 91–100
ФЕМТОСЕКУНДНАЯ СПЕКТРОСКОПИЯ ФОРМИРОВАНИЯ СВОБОДНЫХ ПОЛЯРОНОВ И ПИКОМЕТРОВЫХ ПЕРЕМЕЩЕНИЙ ПРИМЕСНЫХ ИОНОВ В КРИСТАЛЛЕ ФТОРИДА КАДМИЯ
Экспериментально изучена кинетика спектров фотоиндуцированного поглощения кристаллов CdF2 с бистабильными центрами индия и галлия при фемтосекундном импульсном возбуждении. На примере ионов индия показано, что полоса просветления в спектре поглощения глубоких центров формируется в течение времени 0.8–1 пс, что значительно превосходит интервал, в течение которого происходит поглощение фотонов.
Предложена интерпретация этого процесса как результата перемещения иона индия из исходного межузельного положения в узел соседней кристаллической ячейки, дана оценка скорости такого перемещения: 200–250 м/с, что близко к тепловой скорости данного иона при комнатной температуре. Впервые дана экспериментальная оценка времен, характеризующих процесс формирования свободных поляронов вследствие смещения окружающих ионов кристаллической решетки (0.8–1.2 пс).
Оценены времена захвата свободных поляронов трехвалентными ионами галлия и индия, составляющие, соответственно, 5 и 10 пс, а также присущие этим захватам сечения: 2⋅10−16 и 8⋅10−16 см2 соответственно.
Ключевые слова: фемтосекундная спектроскопия.
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